Badlands National Park is approximately 1.5 hours from Mount Rushmore. Take I-90 east towards Wall, SD, to exit 110 or 131 to access Hwy 240's Badlands Loop Road. Check their website for additional information.
While visiting the Badlands you might also want to visit the Minuteman Missile National Historic Site. Visitors can get an upclose look at an intercontinental ballistic missile and be guided through the underground launch control facility. Check their website for additional information.
If you are heading west from Mount Rushmore approximately 2.5 hours away is Devils Tower National Monument. travel west on I-90, exit at Sundance, WY, take Hwy 14 north to Hwy 24 and then take 24 north to Devils Tower. Check their website for additional information.